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• W4200334512 abstract "An enantioselective approach for synthesizing fluorinated azaarenes containing vicinal quaternary-tertiary stereocenters is summarized. The chiral copper(I)-phosphine complex binds with the azaarenes followed by Michael addition to unsaturated acyl imidazoles, resulting in α-functionalized products with an excellent level of enantioselectivities (up to 99%), diastereoselectivities (>20:1), and yields (up to 97%). Furthermore, post-functionalization of the acyl imidazole part has also been demonstrated." @default.
• W4200334512 created "2021-12-31" @default.
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• W4200334512 date "2021-12-06" @default.
• W4200334512 modified "2023-09-26" @default.
• W4200334512 title "Asymmetric α-Functionalization of 2-Alkyl Azaarenes: Synthesis of Tertiary Fluorides Having Vicinal Stereogenic Centers" @default.
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• W4200334512 doi "https://doi.org/10.1021/acs.orglett.1c03626" @default.
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