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- W4200343171 abstract "Abstract Synthesis of covalent organic frameworks (COFs) with desirable organic units furnishes advanced materials with unique functionalities. As an emerging class of two‐dimensional (2D) COFs, sp 2 ‐carbon‐conjugated COFs provide a facile platform to build highly stable and crystalline porous polymers. Herein, a 2D olefin‐linked COF was prepared by employing nanographene, namely, dibenzo[ hi , st ]ovalene (DBOV), as a building block. The DBOV‐COF exhibits unique ABC‐stacked lattices, enhanced stability, and charge‐carrier mobility of ≈0.6 cm 2 V −1 s −1 inferred from ultrafast terahertz photoconductivity measurements. The ABC‐stacking structure was revealed by the high‐resolution transmission electron microscopy and powder X‐ray diffraction. DBOV‐COF demonstrated remarkable photocatalytic activity in hydroxylation, which was attributed to the exposure of narrow‐energy‐gap DBOV cores in the COF pores, in conjunction with efficient charge transport following light absorption." @default.
- W4200343171 created "2021-12-31" @default.
- W4200343171 creator A5017647814 @default.
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- W4200343171 date "2021-12-16" @default.
- W4200343171 modified "2023-10-07" @default.
- W4200343171 title "A Nanographene‐Based Two‐Dimensional Covalent Organic Framework as a Stable and Efficient Photocatalyst" @default.
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