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- W4200344954 abstract "The ramified lithium dendrite growth and severe volume expansion upon the metallic plating process impede the practical deployment of the lithium metal anode in the energy-dense battery system. In this article, a thin modification layer of the Al-based metal–organic framework (MOF) is carbonized into the mesoporous carbon nanorods (PCRs) with atomically dispersed lithiophilic sites; meanwhile these storage units are structurally reinforced by the in-situ grown carbon nanotubes. The interfacial engineered substrate (Al-PCRs/CNTs-Cu) exhibits an enhanced Li affinity with mitigated nucleation barrier, and thus realizes the long-lifespan up to 1000 h at high-capacity-loading of 8 mAh cm−2. When integrating the modified substrate with LiN0.8Co0.1Mn0.1O2 (NCM-811) (∼10.5 mg cm−2) the cathode in a prelithiated full cell model (2*Li excess), the prototype exhibits a high energy density of 414.38 Wh kg−1 at the highest power density of 1243.14 W kg−1. This dual-functionalized, carbonaceous interfacial layer provides a facile and effective approach to construct the energy/power-dense metallic batteries." @default.
- W4200344954 created "2021-12-31" @default.
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- W4200344954 date "2022-03-01" @default.
- W4200344954 modified "2023-10-03" @default.
- W4200344954 title "Threading the MOF-derived mesoporous carbon host with CNT network: An effective modification layer for high-areal-capacity Li metal anodes" @default.
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- W4200344954 doi "https://doi.org/10.1016/j.cej.2021.134194" @default.
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