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- W4200358429 abstract "South Asian air is among the most polluted in the world, causing premature death of millions and asserting a strong perturbation of the regional climate. A central component is carbon monoxide (CO), which is a key modulator of the oxidizing capacity of the atmosphere and a potent indirect greenhouse gas. While CO concentrations are declining elsewhere, South Asia exhibits an increasing trend for unresolved reasons. In this paper, we use dual-isotope (δ13C and δ18O) fingerprinting of CO intercepted in the South Asian outflow to constrain the relative contributions from primary and secondary CO sources. Results show that combustion-derived primary sources dominate the wintertime continental CO fingerprint (fprimary ∼ 79 ± 4%), significantly higher than the global estimate (fprimary ∼ 55 ± 5%). Satellite-based inventory estimates match isotope-constrained fprimary-CO, suggesting observational convergence in source characterization and a prospect for model-observation reconciliation. This ground-truthing emphasizes the pressing need to mitigate incomplete combustion activities for climate/air quality benefits in South Asia." @default.
- W4200358429 created "2021-12-31" @default.
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- W4200358429 date "2021-12-16" @default.
- W4200358429 modified "2023-10-16" @default.
- W4200358429 title "Observational Evidence of Large Contribution from Primary Sources for Carbon Monoxide in the South Asian Outflow" @default.
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- W4200358429 doi "https://doi.org/10.1021/acs.est.1c05486" @default.
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