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- W4200389626 abstract "Crystal phase is an important parameter that can determine the electronic structure and catalytic properties of catalysts. In this work, we report the crystal phase dependent photo- and electrocatalytic oxygen evolution reaction (OER) performance of CoSe2. In electrocatalytic reaction, we firstly found that CoSe2 with orthorhombic phase (o-CoSe2) showed a higher OER performance than that of CoSe2 with cubic phase (c-CoSe2). In the further exploration of photocatalytic application using Fe2O3 as light harvester and CoSe2 as cocatalysts, o-CoSe2/Fe2O3 can realize the qualitative changes of photocatalytic oxygen evolution performance from 0″ to 1. As contrast, c-CoSe2/Fe2O3 cannot work in photocatalytic oxygen evolution process under the same condition. Experimental and theoretical analysis uncover that, the key factor leading to the crystal phase-dependent performance is the decreased activation barrier of H2O on o-CoSe2 surface. This work opens up an opportunity of correlating the CoSe2 crystal phase with performance in OER." @default.
- W4200389626 created "2021-12-31" @default.
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- W4200389626 date "2022-04-01" @default.
- W4200389626 modified "2023-10-16" @default.
- W4200389626 title "Crystal phase engineering boosted photo-electrochemical kinetics of CoSe2 for oxygen evolution catalysis" @default.
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- W4200389626 doi "https://doi.org/10.1016/j.jcis.2021.12.026" @default.
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