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- W4200416588 abstract "Achieving excellent efficiency to mineralize volatile organic compounds (VOCs) under nonthermal plasma catalysis (NTP-catalysis) systems tremendously relies on the catalyst design. Herein, we report a dual-template strategy for synthesizing a core-shell structured nitrogen-enriched hollow hybrid carbon (N-HHC) by a facile pyrolysis of a Mn-ZIF-8@polydopamine core-shell precursor. N-HHC exhibits a remarkable plasma synergy effect and superior degradation efficiency for toluene (up to 90% with a specific input energy of 281 J/L), excellent CO2 selectivity (>45%), and byproduct-inhibiting capability. Such outstanding functionality of the developed N-HHC is uniquely attributed to its hollow multistage and channeling structure, high concentration of O3-decomposing species (pyrrolic and oxide pyridinic-N), and abundant ZnO active sites. Shedding light on an efficient synthetic strategy for designing an advanced nanocatalyst with enhanced VOC destruction in the NTP-catalysis system, the present results could be extended to design other N-doped metal/metal oxide-decorated hollow porous carbons for environment-related applications." @default.
- W4200416588 created "2021-12-31" @default.
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- W4200416588 date "2021-12-27" @default.
- W4200416588 modified "2023-10-14" @default.
- W4200416588 title "Realizing Toluene Deep Mineralization by Coupling Nonthermal Plasma and Nitrogen-Enriched Hollow Hybrid Carbon" @default.
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- W4200416588 doi "https://doi.org/10.1021/acsami.1c20157" @default.
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