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- W4200417113 abstract "Abstract The terpolymerization of a non‐polar olefin (such as ethylene) and two different polar functional olefins in a controlled fashion is of great interest and importance but has hardly been explored to date. We report for the first time the terpolymerization of ethylene ( E ) and two different methoxyaryl‐substituted propylenes ( A R1 P =hexylanisyl propylene; A R2 P =methoxynaphthyl propylene or methoxypyrenyl propylene) by a half‐sandwich scandium catalyst. The terpolymerization took place in a sequence‐controlled fashion, affording unique multi‐block copolymers composed of two different ethylene ‐ alt ‐ methoxyarylpropylene sequences E‐ alt ‐A R1 P (soft segments) and E‐ alt ‐A R2 P (hard segments) and relatively short ethylene–ethylene ( EE ) blocks (crystalline segments). The terpolymers exhibited excellent elasticity and unprecedented self‐healing as a result of microphase separation of nanodomains of the crystalline EE segments and the hard amorphous E‐ alt ‐A R2 P segments from a very flexible E‐ alt ‐A R1 P matrix, demonstrating unique synergy of the three different components." @default.
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- W4200417113 date "2021-11-09" @default.
- W4200417113 modified "2023-10-14" @default.
- W4200417113 title "Terpolymerization of Ethylene and Two Different Methoxyaryl‐Substituted Propylenes by Scandium Catalyst Makes Tough and Fast Self‐Healing Elastomers" @default.
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- W4200417113 doi "https://doi.org/10.1002/ange.202111161" @default.
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