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• W4200427908 abstract "Metal-free organic perovskites such as [HMDABCO](NH4)I3 ([HMDABCO2+] = 1-methyl-1,4-diazabicyclo[2.2.2]octane-1,4-diium) have recently emerged as sustainable high-performance ferroelectrics. To realize their application as a substitute for metal-based analogues in microelectronic devices, it is mandatory to establish a process for their fabrication in the form of thin films. Here, we investigate different deposition techniques such as spin, spray, and drop coating for their eligibility in the production of crystalline, dense, and smooth [HMDABCO](NH4)I3 thin films. By systematically varying different process parameters, we show how to control the thin-film thickness, influence the preferred crystallite orientation, and obtain dense thin films, which were characterized by grazing incidence X-ray diffraction, scanning electron microscopy, and atomic force microscopy. Our work presents the first deposition of [HMDABCO](NH4)I3 as thin films and provides the experimental and scientific basis for further systematic investigations." @default.
• W4200427908 created "2021-12-31" @default.
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• W4200427908 date "2021-12-14" @default.
• W4200427908 modified "2023-09-26" @default.
• W4200427908 title "Synthetic Approaches Targeting Metal-Free Perovskite [HMDABCO](NH₄)I₃ Thin Films" @default.
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• W4200427908 doi "https://doi.org/10.1021/acs.cgd.1c01042" @default.
• W4200427908 hasPublicationYear "2021" @default.
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