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- W4200440984 abstract "Compromised performance caused by gas product adhesion remains a major challenge for membrane applications in chlor-alkali electrolysis. Here, an ultra-bubble-repellent sodium perfluorosulfonic acid (PFSA-Na) membrane with hierarchical structures of aggregated silica was successfully synthesized by tethering hydrophilic silica onto a mussel-inspired intermediate layer. The surface chemistry, morphology and loading could be controlled via surface tailoring of the silica by γ-(2,3-epoxypropoxy)propyltrimethoxysilane (KH560). The developed membrane exhibited high hydrophilicity (7.5 ± 1.3°), an ultralow bubble contact area (164.7 ± 2.1°) and negligible bubble adhesion forces (<6 μN) while maintaining efficient NaCl transport and low electric double layer resistance. The superaerophobic-hydrophilic surface enables an excellent cleaning property. When the modified membrane was applied in chlor-alkali electrolysis, the Cl2/H2 gas bubbles were repelled from the membrane surface in time and minimized the negative effects of bubble adhesion, resulting in high-efficiency chlor-alkali electrolysis. Further, the developed membrane exhibited high stability during the continuous 10-h electrolysis process. This result indicates that developing a superaerophobic surface with highly efficient mass transport can lead to high-performance chlor-alkali electrolysis." @default.
- W4200440984 created "2021-12-31" @default.
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- W4200440984 date "2022-02-01" @default.
- W4200440984 modified "2023-10-16" @default.
- W4200440984 title "Ultra-bubble-repellent sodium perfluorosulfonic acid membrane with a mussel-inspired intermediate layer for high-efficiency chlor-alkali electrolysis" @default.
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- W4200440984 doi "https://doi.org/10.1016/j.memsci.2021.120181" @default.
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