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• W4200453212 abstract "Electrochemical reduction of CO2 to value-added chemicals holds promise for carbon utilization and renewable electricity storage. However, selective CO2 reduction to multi-carbon fuels remains a significant challenge. Here, we report that B/N-doped sp3/sp2 hybridized nanocarbon (BNHC), consisting of ultra-small nanoparticles with a sp3 carbon core covered by a sp2 carbon shell, is an efficient electrocatalyst for electrochemical reduction of CO2 to ethanol at relatively low overpotentials. CO2 reduction occurs with a Faradaic efficiency of 58.8%-69.1% for ethanol and acetate production at −0.5 ∼ −0.6 V (vs. RHE), among which 51.6%-56.0% is for ethanol. The high selectivity for ethanol is due to the integrated effect of sp3/sp2 carbon and B/N doping. Both sp3 carbon and B/N doping contribute to enhanced ethanol production with sp2 carbon reducing the overpotential for CO2 reduction to ethanol." @default.
• W4200453212 created "2021-12-31" @default.
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• W4200453212 date "2022-10-01" @default.
• W4200453212 modified "2023-10-03" @default.
• W4200453212 title "Promoting electrochemical reduction of CO2 to ethanol by B/N-doped sp3/sp2 nanocarbon electrode" @default.
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• W4200453212 doi "https://doi.org/10.1016/j.cclet.2021.12.063" @default.
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