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- W4200490463 abstract "Here, six phenanthrene (the smallest arm-chair graphene nanoribbon) derivatives with dithiomethyl substitutions at different positions as the anchoring groups were synthesized. Scanning tunneling microscopy break junction technique was used to measure their single molecule conductances between gold electrodes, which showed a difference as much as 20-fold in the range of ∼10-2.82 G0 to ∼10-4.09 G0 following the trend of G2,7 > G3,6 > G2,6 > G1,7 > G1,6 > G1,8. DFT calculations agree well with this measured trend and indicate that the single molecule conductances are a combination of energy alignment, electronic coupling, and quantum effects. This significant regio- and steric effect on the single molecule conductance of phenanthrene model molecules shows the complexity in the practice of graphene nanoribbons as building blocks for future carbon-based electronics in one hand but also provides good conductance tunability on the other hand." @default.
- W4200490463 created "2021-12-31" @default.
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- W4200490463 date "2021-12-07" @default.
- W4200490463 modified "2023-10-16" @default.
- W4200490463 title "Regio- and Steric Effects on Single Molecule Conductance of Phenanthrenes" @default.
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- W4200490463 doi "https://doi.org/10.1021/acs.nanolett.1c03565" @default.
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