Matches in SemOpenAlex for { <https://semopenalex.org/work/W4200496433> ?p ?o ?g. }
- W4200496433 abstract "Metal organic frameworks (MOFs) and corresponding derivatives have attracted wide attention. As electrocatalysts, these derivatives (metal, metal compound, and associated composites) have a wide range of application in water-splitting devices, fuel cells, and other hydrogen-related technologies. However, with the exception of pyrolysis, limited studies have documented generated metal nanoparticles from MOFs hydrolysis reactions. Herein, NiRu dual-phase alloy nanoparticles are synthesized via in situ MOFs hydrolysis mediating solvothermal reduction reaction. The hcp-phase NiRu alloys can be rationally tuned by modulating experimental parameters of feeding metal ratio and reaction time. The volcanic link between hydrogen evolution reaction activity and the descriptor of d band center is investigated using experimentally determined valence bands. Furthermore, compared with fcc-phase NiRu alloys, it is theoretically revealed that hcp-phase NiRu alloys optimize d band structure and have a lower energy barrier. This finding broadens the range of application for MOFs hydrolysis reactions and highlights advantages of metal alloys manufactured from MOFs hydrolysis reactions." @default.
- W4200496433 created "2021-12-31" @default.
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- W4200496433 date "2021-12-22" @default.
- W4200496433 modified "2023-10-17" @default.
- W4200496433 title "Tuning Phase Structure of Nickel–Ruthenium Alloys via MOFs In Situ Hydrolysis toward Enhanced Hydrogen Evolution Performance in Alkaline" @default.
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- W4200496433 doi "https://doi.org/10.1002/smtd.202101188" @default.
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