Matches in SemOpenAlex for { <https://semopenalex.org/work/W4200523923> ?p ?o ?g. }
- W4200523923 abstract "Photocatalytic synthesis of ammonia (NH3 ) holds significant potential compared with the Haber-Bosch process. However, the reported photocatalysts suffer from low efficiency owing to localized electron deficiency. Herein, Ru-SA (single atoms)/Hx MoO3-y hybrids with abundant of Mon+ (4<n<6) species neighboring oxygen vacancies (OV ) are synthesized via a H-spillover process. Detailed characterizations demonstrate that Ru-SA/Hx MoO3-y hybrids can quantitatively produce NH3 from N2 and H2 through the presence of dual active centers (Ru SA and Mon+ ). The Ru SA boost the activation and migration of H2 , and Mon+ species act as the trapping sites of localized electrons and the adsorption and dissociation sites of N2 , finally leading to NH3 synthesis on Mon+ -OH. The NH3 generation rate is up to 4.0 mmol h-1 g-1 , accompanied by an apparent quantum efficiency over 6.0 % at 650 nm." @default.
- W4200523923 created "2021-12-31" @default.
- W4200523923 creator A5007477535 @default.
- W4200523923 creator A5013501735 @default.
- W4200523923 creator A5028494580 @default.
- W4200523923 creator A5050100282 @default.
- W4200523923 creator A5063483273 @default.
- W4200523923 creator A5074920133 @default.
- W4200523923 date "2022-02-10" @default.
- W4200523923 modified "2023-10-14" @default.
- W4200523923 title "Dual Active Centers Bridged by Oxygen Vacancies of Ruthenium Single‐Atom Hybrids Supported on Molybdenum Oxide for Photocatalytic Ammonia Synthesis" @default.
- W4200523923 cites W1238502700 @default.
- W4200523923 cites W1853517821 @default.
- W4200523923 cites W1972901386 @default.
- W4200523923 cites W1992023766 @default.
- W4200523923 cites W1997721562 @default.
- W4200523923 cites W2015664999 @default.
- W4200523923 cites W2020023668 @default.
- W4200523923 cites W2028510889 @default.
- W4200523923 cites W2038851518 @default.
- W4200523923 cites W2044766600 @default.
- W4200523923 cites W2048074758 @default.
- W4200523923 cites W2048110396 @default.
- W4200523923 cites W2048703881 @default.
- W4200523923 cites W2052606906 @default.
- W4200523923 cites W2060437361 @default.
- W4200523923 cites W2070377341 @default.
- W4200523923 cites W2090749185 @default.
- W4200523923 cites W2091557431 @default.
- W4200523923 cites W2093495583 @default.
- W4200523923 cites W2097378387 @default.
- W4200523923 cites W2108670893 @default.
- W4200523923 cites W2165882368 @default.
- W4200523923 cites W2276551461 @default.
- W4200523923 cites W2315707420 @default.
- W4200523923 cites W2325627160 @default.
- W4200523923 cites W2462520899 @default.
- W4200523923 cites W2510877666 @default.
- W4200523923 cites W2581400290 @default.
- W4200523923 cites W2604447493 @default.
- W4200523923 cites W2604794936 @default.
- W4200523923 cites W2626655409 @default.
- W4200523923 cites W2687572373 @default.
- W4200523923 cites W2736305270 @default.
- W4200523923 cites W2750205897 @default.
- W4200523923 cites W2768860599 @default.
- W4200523923 cites W2781135986 @default.
- W4200523923 cites W2794256365 @default.
- W4200523923 cites W2854019328 @default.
- W4200523923 cites W2910746619 @default.
- W4200523923 cites W2919173788 @default.
- W4200523923 cites W2942802063 @default.
- W4200523923 cites W2969516292 @default.
- W4200523923 cites W2970514418 @default.
- W4200523923 cites W2976438310 @default.
- W4200523923 cites W3015003454 @default.
- W4200523923 cites W3027257336 @default.
- W4200523923 cites W3027504699 @default.
- W4200523923 cites W3087027651 @default.
- W4200523923 cites W3096007721 @default.
- W4200523923 cites W3097543460 @default.
- W4200523923 cites W3097930019 @default.
- W4200523923 cites W3169660990 @default.
- W4200523923 cites W4231646636 @default.
- W4200523923 cites W4242214373 @default.
- W4200523923 cites W4251642750 @default.
- W4200523923 doi "https://doi.org/10.1002/anie.202114242" @default.
- W4200523923 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34918452" @default.
- W4200523923 hasPublicationYear "2022" @default.
- W4200523923 type Work @default.
- W4200523923 citedByCount "32" @default.
- W4200523923 countsByYear W42005239232022 @default.
- W4200523923 countsByYear W42005239232023 @default.
- W4200523923 crossrefType "journal-article" @default.
- W4200523923 hasAuthorship W4200523923A5007477535 @default.
- W4200523923 hasAuthorship W4200523923A5013501735 @default.
- W4200523923 hasAuthorship W4200523923A5028494580 @default.
- W4200523923 hasAuthorship W4200523923A5050100282 @default.
- W4200523923 hasAuthorship W4200523923A5063483273 @default.
- W4200523923 hasAuthorship W4200523923A5074920133 @default.
- W4200523923 hasConcept C102931765 @default.
- W4200523923 hasConcept C147789679 @default.
- W4200523923 hasConcept C161790260 @default.
- W4200523923 hasConcept C178790620 @default.
- W4200523923 hasConcept C179104552 @default.
- W4200523923 hasConcept C181258405 @default.
- W4200523923 hasConcept C185592680 @default.
- W4200523923 hasConcept C2776382133 @default.
- W4200523923 hasConcept C2779851234 @default.
- W4200523923 hasConcept C540031477 @default.
- W4200523923 hasConcept C549387045 @default.
- W4200523923 hasConcept C555196967 @default.
- W4200523923 hasConcept C65165184 @default.
- W4200523923 hasConcept C75473681 @default.
- W4200523923 hasConceptScore W4200523923C102931765 @default.
- W4200523923 hasConceptScore W4200523923C147789679 @default.
- W4200523923 hasConceptScore W4200523923C161790260 @default.
- W4200523923 hasConceptScore W4200523923C178790620 @default.
- W4200523923 hasConceptScore W4200523923C179104552 @default.
- W4200523923 hasConceptScore W4200523923C181258405 @default.