FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4200552747> ?p ?o ?g. }

• W4200552747 endingPage "4661" @default.
• W4200552747 startingPage "4653" @default.
• W4200552747 abstract "Developing efficient catalysts of low-cost transition metals for hydrogen production is of great importance but remains a huge challenge. Motivated by the idea of engineering local atomic configuration, we propose to focus on single metal atom confined in the lattice oxygen environment, as a class of non-Pt catalysts for hydrogen production. By first principles calculations, we study the characteristics and mechanism of hydrogen evolution reaction of single-atom Cu supported on anatase TiO2 catalysts, Cu1/TiO2. Cu preferentially sits on the bridge-centre site between two 2-fold coordinated O atoms (O2c) on the surface. Cu and coordinated O2c function as copper oxide species (-Cu-O-) in the reaction. The reaction starts with two isolated H respectively positioned on Cu and O2c, proceeds with a transfer of H from O2c to Cu, and eventually forms a H2 molecule. The free energy profiles indicate that Cu1/TiO2 exhibits excellent hydrogen evolution activity even better than Pt and MoS2. This study not only shows that single-atom Cu1/TiO2 is an excellent hydrogen evolution catalyst, but also expands the understanding of oxide species in single-atom catalysis and proposes an engineering local atomic configuration strategy for optimizing the design of single-atom catalysts for enhanced hydrogen production." @default.
• W4200552747 created "2021-12-31" @default.
• W4200552747 creator A5006947678 @default.
• W4200552747 creator A5019053282 @default.
• W4200552747 creator A5023591114 @default.
• W4200552747 creator A5056340751 @default.
• W4200552747 date "2022-01-01" @default.
• W4200552747 modified "2023-10-02" @default.
• W4200552747 title "Insight into enhanced hydrogen evolution of single-atom Cu1/TiO2 catalysts from first principles" @default.
• W4200552747 cites W1487506519 @default.
• W4200552747 cites W1816450589 @default.
• W4200552747 cites W1966156734 @default.
• W4200552747 cites W1968748900 @default.
• W4200552747 cites W1969174174 @default.
• W4200552747 cites W1970127494 @default.
• W4200552747 cites W1972673502 @default.
• W4200552747 cites W1973891115 @default.
• W4200552747 cites W1977700257 @default.
• W4200552747 cites W1979371521 @default.
• W4200552747 cites W1979544533 @default.
• W4200552747 cites W1979778096 @default.
• W4200552747 cites W1989029881 @default.
• W4200552747 cites W1990190733 @default.
• W4200552747 cites W1990207931 @default.
• W4200552747 cites W1991149034 @default.
• W4200552747 cites W2004809223 @default.
• W4200552747 cites W2007395042 @default.
• W4200552747 cites W2009734832 @default.
• W4200552747 cites W2018651936 @default.
• W4200552747 cites W2021318889 @default.
• W4200552747 cites W2022714449 @default.
• W4200552747 cites W2022817821 @default.
• W4200552747 cites W2031430816 @default.
• W4200552747 cites W2033256351 @default.
• W4200552747 cites W2036113194 @default.
• W4200552747 cites W2041322147 @default.
• W4200552747 cites W2041606536 @default.
• W4200552747 cites W2042492216 @default.
• W4200552747 cites W2055261628 @default.
• W4200552747 cites W2065922993 @default.
• W4200552747 cites W2077822985 @default.
• W4200552747 cites W2082788869 @default.
• W4200552747 cites W2083222334 @default.
• W4200552747 cites W2083626135 @default.
• W4200552747 cites W2084024698 @default.
• W4200552747 cites W2091633783 @default.
• W4200552747 cites W2092604148 @default.
• W4200552747 cites W2109002260 @default.
• W4200552747 cites W2122427541 @default.
• W4200552747 cites W2128255830 @default.
• W4200552747 cites W2132316147 @default.
• W4200552747 cites W2133795748 @default.
• W4200552747 cites W2133879494 @default.
• W4200552747 cites W2151800339 @default.
• W4200552747 cites W2160151078 @default.
• W4200552747 cites W2324576880 @default.
• W4200552747 cites W2337970968 @default.
• W4200552747 cites W2421882692 @default.
• W4200552747 cites W2465500435 @default.
• W4200552747 cites W2575316286 @default.
• W4200552747 cites W2617194355 @default.
• W4200552747 cites W2790522882 @default.
• W4200552747 cites W2801820474 @default.
• W4200552747 cites W2901911184 @default.
• W4200552747 cites W2906521174 @default.
• W4200552747 cites W2912908023 @default.
• W4200552747 cites W2922281588 @default.
• W4200552747 cites W2936791207 @default.
• W4200552747 cites W2963476952 @default.
• W4200552747 cites W2990136355 @default.
• W4200552747 cites W3008901732 @default.
• W4200552747 cites W3016888219 @default.
• W4200552747 cites W3084070160 @default.
• W4200552747 doi "https://doi.org/10.1016/j.ijhydene.2021.11.115" @default.
• W4200552747 hasPublicationYear "2022" @default.
• W4200552747 type Work @default.
• W4200552747 citedByCount "10" @default.
• W4200552747 countsByYear W42005527472022 @default.
• W4200552747 countsByYear W42005527472023 @default.
• W4200552747 crossrefType "journal-article" @default.
• W4200552747 hasAuthorship W4200552747A5006947678 @default.
• W4200552747 hasAuthorship W4200552747A5019053282 @default.
• W4200552747 hasAuthorship W4200552747A5023591114 @default.
• W4200552747 hasAuthorship W4200552747A5056340751 @default.
• W4200552747 hasConcept C106773901 @default.
• W4200552747 hasConcept C147789679 @default.
• W4200552747 hasConcept C149635348 @default.
• W4200552747 hasConcept C159467904 @default.
• W4200552747 hasConcept C161790260 @default.
• W4200552747 hasConcept C171250308 @default.
• W4200552747 hasConcept C178790620 @default.
• W4200552747 hasConcept C179104552 @default.
• W4200552747 hasConcept C185592680 @default.
• W4200552747 hasConcept C192562407 @default.
• W4200552747 hasConcept C202189072 @default.
• W4200552747 hasConcept C2776640939 @default.
• W4200552747 hasConcept C2779851234 @default.
• W4200552747 hasConcept C2780263894 @default.

• next