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- W4200552756 endingPage "3995" @default.
- W4200552756 startingPage "3966" @default.
- W4200552756 abstract "Direct conversion of methane to C2 compounds by oxidative and nonoxidative coupling reactions has been intensively studied in the past four decades; however, because these reactions have intrinsic severe thermodynamic constraints, they have not become viable industrially. Recently, with the increasing availability of inexpensive green electrons coming from renewable sources, electrochemical technologies are gaining momentum for reactions that have been challenging for more conventional catalysis. Using solid-state membranes to control the reacting species and separate products in a single step is a crucial advantage. Devices using ionic or mixed ionic-electronic conductors can be explored for methane coupling reactions with great potential to increase selectivity. Although these technologies are still in the early scaling stages, they offer a sustainable path for the utilization of methane and benefit from the advances in both solid oxide fuel cells and electrolyzers. This review identifies promising developments for solid-state methane conversion reactors by assessing multifunctional layers with microstructural control; combining solid electrolytes (proton and oxygen ion conductors) with active and selective electrodes/catalysts; applying more efficient reactor designs; understanding the reaction/degradation mechanisms; defining standards for performance evaluation; and carrying techno-economic analysis." @default.
- W4200552756 created "2021-12-31" @default.
- W4200552756 creator A5024211746 @default.
- W4200552756 creator A5026299634 @default.
- W4200552756 creator A5046965156 @default.
- W4200552756 creator A5051496511 @default.
- W4200552756 creator A5091089592 @default.
- W4200552756 date "2021-12-28" @default.
- W4200552756 modified "2023-10-17" @default.
- W4200552756 title "Direct Conversion of Methane to C<sub>2</sub> Hydrocarbons in Solid-State Membrane Reactors at High Temperatures" @default.
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