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- W4200560869 abstract "Engineering of advanced, highly efficient, and stable nanomaterials to load more recognition units and effectively accelerate gas adsorption and diffusion is desired. To this end, in this work, palladium (Pd)@titanium dioxide (TiO2)/carbon nitride nanosheet (C3N4) ternary heterostructure sensing materials were synthesized by using the combinational methodology of solvothermal growth and calcination. The characterization elucidated the successful formation of [email protected]2 core-shell nanoparticles on the surface of C3N4 nanosheets. The gas sensing properties of [email protected]2/C3N4 heterostructures with different mass ratios of Pd were examined. The experimental results showed that the fabricated 5% [email protected]2/C3N4 sensor exhibits a high ethanol response value in a wide concentration range (50–10000 ppm), a short response time (30 s) with fast recovery property (15 s), high selectivity toward ethanol, and excellent stability at 125 °C. The remarkably enhanced sensing performance of the ternary [email protected]2/C3N4 heterostructure is on account of chemical as well as electronic sensitization of Pd nanoparticles, n-n heterojunction formation, and the 2D layered structure of the C3N4 assisting the charge transfer. The present findings are expected to provide inspirational insights into the design and fabrication of highly sensitive gas sensors." @default.
- W4200560869 created "2021-12-31" @default.
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- W4200560869 date "2022-04-01" @default.
- W4200560869 modified "2023-09-25" @default.
- W4200560869 title "Introducing efficient and stable Palladium@Titanium dioxide/carbon nitride nanosheet: Accelerating surface reactions for the selective detection of ethanol in a wide concentration range" @default.
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- W4200560869 doi "https://doi.org/10.1016/j.ceramint.2021.12.184" @default.
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