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- W4200573885 abstract "Abstract Although multiple oxide-based solid electrolyte materials with intrinsically high ionic conductivities have emerged, practical processing and synthesis routes introduce grain boundaries and other interfaces that can perturb primary conduction channels. To directly probe these effects, we demonstrate an efficient and general mesoscopic computational method capable of predicting effective ionic conductivity through a complex polycrystalline oxide-based solid electrolyte microstructure without relying on simplified equivalent circuit description. We parameterize the framework for Li 7- x La 3 Zr 2 O 12 (LLZO) garnet solid electrolyte by combining synthetic microstructures from phase-field simulations with diffusivities from molecular dynamics simulations of ordered and disordered systems. Systematically designed simulations reveal an interdependence between atomistic and mesoscopic microstructural impacts on the effective ionic conductivity of polycrystalline LLZO, quantified by newly defined metrics that characterize the complex ionic transport mechanism. Our results provide fundamental understanding of the physical origins of the reported variability in ionic conductivities based on an extensive analysis of literature data, while simultaneously outlining practical design guidance for achieving desired ionic transport properties based on conditions for which sensitivity to microstructural features is highest. Additional implications of our results are discussed, including a possible connection between ion conduction behavior and dendrite formation." @default.
- W4200573885 created "2021-12-31" @default.
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- W4200573885 date "2021-12-21" @default.
- W4200573885 modified "2023-10-17" @default.
- W4200573885 title "Microstructural impacts on ionic conductivity of oxide solid electrolytes from a combined atomistic-mesoscale approach" @default.
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- W4200573885 cites W1965764022 @default.
- W4200573885 cites W1973759826 @default.
- W4200573885 cites W1978362245 @default.
- W4200573885 cites W1985361961 @default.
- W4200573885 cites W1988158958 @default.
- W4200573885 cites W1996879303 @default.
- W4200573885 cites W1998937828 @default.
- W4200573885 cites W2002723646 @default.
- W4200573885 cites W2005912108 @default.
- W4200573885 cites W2007641411 @default.
- W4200573885 cites W2012284610 @default.
- W4200573885 cites W2013605392 @default.
- W4200573885 cites W2017265410 @default.
- W4200573885 cites W2019465613 @default.
- W4200573885 cites W2034286146 @default.
- W4200573885 cites W2041001120 @default.
- W4200573885 cites W2041368213 @default.
- W4200573885 cites W2042203745 @default.
- W4200573885 cites W2043701535 @default.
- W4200573885 cites W2046528357 @default.
- W4200573885 cites W2064146245 @default.
- W4200573885 cites W2068157181 @default.
- W4200573885 cites W2079653074 @default.
- W4200573885 cites W2085039336 @default.
- W4200573885 cites W2121636359 @default.
- W4200573885 cites W2122589748 @default.
- W4200573885 cites W2126027377 @default.
- W4200573885 cites W2132820239 @default.
- W4200573885 cites W2138805126 @default.
- W4200573885 cites W2143795526 @default.
- W4200573885 cites W2152048732 @default.
- W4200573885 cites W2157912828 @default.
- W4200573885 cites W2166330692 @default.
- W4200573885 cites W2174287776 @default.
- W4200573885 cites W2197550433 @default.
- W4200573885 cites W2265416121 @default.
- W4200573885 cites W227761974 @default.
- W4200573885 cites W2310846280 @default.
- W4200573885 cites W2313515426 @default.
- W4200573885 cites W2333986953 @default.
- W4200573885 cites W2345398523 @default.
- W4200573885 cites W2398528971 @default.
- W4200573885 cites W2504274499 @default.
- W4200573885 cites W2560348663 @default.
- W4200573885 cites W2601177278 @default.
- W4200573885 cites W2752563240 @default.
- W4200573885 cites W2753662284 @default.
- W4200573885 cites W2765540043 @default.
- W4200573885 cites W2765760561 @default.
- W4200573885 cites W2775058775 @default.
- W4200573885 cites W2789489435 @default.
- W4200573885 cites W2791537261 @default.
- W4200573885 cites W2793872957 @default.
- W4200573885 cites W2795226759 @default.
- W4200573885 cites W2799522686 @default.
- W4200573885 cites W2884213676 @default.
- W4200573885 cites W2884363481 @default.
- W4200573885 cites W2888420309 @default.
- W4200573885 cites W2890258988 @default.
- W4200573885 cites W2895989477 @default.
- W4200573885 cites W2900429435 @default.
- W4200573885 cites W2903195550 @default.
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- W4200573885 cites W2913909639 @default.
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- W4200573885 cites W2918721424 @default.
- W4200573885 cites W2947619044 @default.
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- W4200573885 cites W2969542859 @default.
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- W4200573885 cites W3018657932 @default.
- W4200573885 cites W3021828269 @default.
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- W4200573885 doi "https://doi.org/10.1038/s41524-021-00681-8" @default.
- W4200573885 hasPublicationYear "2021" @default.
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