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- W4200600049 startingPage "139769" @default.
- W4200600049 abstract "Solid-state lithium metal batteries (SSLMBs) are considered as a promising energy storage technology due to their high energy density and safety. However, the relatively low conductivity of solid-state electrolytes and the high electrolyte–electrode interfacial resistance seriously limited the development of SSLMBs. In this work, the high-performance PEO-based composite polymer electrolyte (3D CPE-5) was successfully prepared by reinforcing with polyvinylidene fluoride–hexafluoropropylene nanofibers and Li1.3Al0.3Ti1.7(PO4)3 (LATP) particles. The thickness of 3D CPE-5 is only 50 μm with high electrochemical window (5.21 V) and lithium transference number (0.49) at 60 ℃. In addition, the 3D CPE-5 shows excellent stability to Li–metal, so that Li–Li symmetric cells can run stably for more than 300 h under 0.1 mA cm−2 with low voltage polarization value (15 mV) and effective lithium dendrite inhibition. Finally, the high-voltage Li/3D CPE-5/NCM811 (LiNi0.8Co0.1Mn0.1O2) solid-state battery demonstrates excellent cycling stability at 0.1 and 0.5 C (60 ℃). The excellent safety performance of 3D CPE-5 highlights its remarkable advantages over liquid electrolytes and provide an effective design strategy of high-performance polymer electrolytes for SSLMBs." @default.
- W4200600049 created "2021-12-31" @default.
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- W4200600049 date "2022-02-01" @default.
- W4200600049 modified "2023-10-05" @default.
- W4200600049 title "3D poly(vinylidene fluoride–hexafluoropropylen) nanofiber-reinforced PEO-based composite polymer electrolyte for high-voltage lithium metal batteries" @default.
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- W4200600049 doi "https://doi.org/10.1016/j.electacta.2021.139769" @default.
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