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- W4200604801 endingPage "26191" @default.
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- W4200604801 abstract "Abstract Selective molecular recognition in water is the foundation of numerous biological functions but is a challenge for most synthetic hosts. We employ the concept of endo‐functionalized cavity and the strategy of simultaneous construction to address this issue. The concept and the strategy were demonstrated in the construction of a biomimetic host for selectively recognizing quinones in water. The host was synthesized by joining two pieces of bent anthracene dimer through amide bond formation, affording a deep hydrophobic cavity and inward‐directing hydrogen bonding sites. The host can recognize quinones over their close analogues in water, and its association affinity to p‐benzoquinone is the highest among all the known hosts and is even comparable to that of the bioreceptor. The binding with an anthraquinone reaches nanomolar affinity. Shielded hydrogen bonding, C−H⋅⋅⋅π, and charge transfer interactions, and the hydrophobic effect are responsible for the high binding affinity and selectivity." @default.
- W4200604801 created "2021-12-31" @default.
- W4200604801 creator A5013813264 @default.
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- W4200604801 creator A5071464070 @default.
- W4200604801 creator A5087709746 @default.
- W4200604801 creator A5089812226 @default.
- W4200604801 date "2021-11-02" @default.
- W4200604801 modified "2023-10-14" @default.
- W4200604801 title "Biomimetic Recognition of Quinones in Water by an <i>Endo</i>‐Functionalized Cavity with Anthracene Sidewalls" @default.
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- W4200604801 doi "https://doi.org/10.1002/ange.202112267" @default.
- W4200604801 hasPublicationYear "2021" @default.