FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4200605890> ?p ?o ?g. }

• W4200605890 endingPage "4384" @default.
• W4200605890 startingPage "4380" @default.
• W4200605890 abstract "Carbon dioxide electrochemical reduction (CO2RR) has been recognized as an efficient way to mitigate CO2 emissions and alleviate the pressure on global warming and associated environmental consequences. Gold (Au) is reported as stable and active electrocatalysts to convert CO2 to CO at low overpotential due to its moderate adsorption strength of *COOH and *CO. The request for improved catalytic performance, however, is motivated by current unsatisfied catalytic selectivity because of the side hydrogen evolution reaction. In this context, the design of Au based binary catalysts that can boost CO selectivity is of great interest. In the present work, we report that Au nanoparticles can be feasibly dispersed and anchored on silicon nanowires to form Au-Si binary nanomaterials. The Au-Si may stably drive CO2RR with a CO Faraday efficiency of 95.6% at −0.6 V vs. RHE in 0.5 mol/L KHCO3 solution. Such selectivity outperforms Au particles by up to 61%. Controlled experiments illustrate that such catalytic enhancement can chiefly be ascribed to electronic effects of binary catalysts. Theoretical calculations reveal that spontaneously produced silicon oxide may not only inhibit hydrogen evolution reaction, but also stabilize the key intermediate *COOH in CO formation." @default.
• W4200605890 created "2021-12-31" @default.
• W4200605890 creator A5018624308 @default.
• W4200605890 creator A5021658618 @default.
• W4200605890 creator A5026077382 @default.
• W4200605890 creator A5035944985 @default.
• W4200605890 creator A5043301652 @default.
• W4200605890 creator A5053780153 @default.
• W4200605890 creator A5057299366 @default.
• W4200605890 creator A5071238079 @default.
• W4200605890 creator A5074338325 @default.
• W4200605890 date "2022-09-01" @default.
• W4200605890 modified "2023-10-09" @default.
• W4200605890 title "Boosting electrocatalytic selectivity in carbon dioxide reduction: The fundamental role of dispersing gold nanoparticles on silicon nanowires" @default.
• W4200605890 cites W2060441729 @default.
• W4200605890 cites W2160252043 @default.
• W4200605890 cites W2297401062 @default.
• W4200605890 cites W2334092527 @default.
• W4200605890 cites W2336959805 @default.
• W4200605890 cites W2436645641 @default.
• W4200605890 cites W2494233754 @default.
• W4200605890 cites W2496132953 @default.
• W4200605890 cites W2611930531 @default.
• W4200605890 cites W2614522003 @default.
• W4200605890 cites W2680128116 @default.
• W4200605890 cites W2725997949 @default.
• W4200605890 cites W2795259398 @default.
• W4200605890 cites W2886103182 @default.
• W4200605890 cites W2911533935 @default.
• W4200605890 cites W2913280791 @default.
• W4200605890 cites W2936610288 @default.
• W4200605890 cites W2943377328 @default.
• W4200605890 cites W2944984983 @default.
• W4200605890 cites W2965483738 @default.
• W4200605890 cites W2995730492 @default.
• W4200605890 cites W3005814135 @default.
• W4200605890 cites W3034624833 @default.
• W4200605890 cites W3093108767 @default.
• W4200605890 cites W3104917636 @default.
• W4200605890 cites W3113344131 @default.
• W4200605890 cites W3120746273 @default.
• W4200605890 cites W3132750624 @default.
• W4200605890 cites W3133189482 @default.
• W4200605890 cites W3147780002 @default.
• W4200605890 cites W3153839205 @default.
• W4200605890 cites W3165216038 @default.
• W4200605890 cites W764408565 @default.
• W4200605890 doi "https://doi.org/10.1016/j.cclet.2021.12.034" @default.
• W4200605890 hasPublicationYear "2022" @default.
• W4200605890 type Work @default.
• W4200605890 citedByCount "4" @default.
• W4200605890 countsByYear W42006058902023 @default.
• W4200605890 crossrefType "journal-article" @default.
• W4200605890 hasAuthorship W4200605890A5018624308 @default.
• W4200605890 hasAuthorship W4200605890A5021658618 @default.
• W4200605890 hasAuthorship W4200605890A5026077382 @default.
• W4200605890 hasAuthorship W4200605890A5035944985 @default.
• W4200605890 hasAuthorship W4200605890A5043301652 @default.
• W4200605890 hasAuthorship W4200605890A5053780153 @default.
• W4200605890 hasAuthorship W4200605890A5057299366 @default.
• W4200605890 hasAuthorship W4200605890A5071238079 @default.
• W4200605890 hasAuthorship W4200605890A5074338325 @default.
• W4200605890 hasConcept C118792377 @default.
• W4200605890 hasConcept C127413603 @default.
• W4200605890 hasConcept C138631740 @default.
• W4200605890 hasConcept C147789679 @default.
• W4200605890 hasConcept C155672457 @default.
• W4200605890 hasConcept C161790260 @default.
• W4200605890 hasConcept C171250308 @default.
• W4200605890 hasConcept C17525397 @default.
• W4200605890 hasConcept C178790620 @default.
• W4200605890 hasConcept C179104552 @default.
• W4200605890 hasConcept C185592680 @default.
• W4200605890 hasConcept C186460083 @default.
• W4200605890 hasConcept C191897082 @default.
• W4200605890 hasConcept C192562407 @default.
• W4200605890 hasConcept C24596552 @default.
• W4200605890 hasConcept C42360764 @default.
• W4200605890 hasConcept C512735826 @default.
• W4200605890 hasConcept C512968161 @default.
• W4200605890 hasConcept C52859227 @default.
• W4200605890 hasConcept C544956773 @default.
• W4200605890 hasConcept C55904794 @default.
• W4200605890 hasConcept C74214498 @default.
• W4200605890 hasConceptScore W4200605890C118792377 @default.
• W4200605890 hasConceptScore W4200605890C127413603 @default.
• W4200605890 hasConceptScore W4200605890C138631740 @default.
• W4200605890 hasConceptScore W4200605890C147789679 @default.
• W4200605890 hasConceptScore W4200605890C155672457 @default.
• W4200605890 hasConceptScore W4200605890C161790260 @default.
• W4200605890 hasConceptScore W4200605890C171250308 @default.
• W4200605890 hasConceptScore W4200605890C17525397 @default.
• W4200605890 hasConceptScore W4200605890C178790620 @default.
• W4200605890 hasConceptScore W4200605890C179104552 @default.
• W4200605890 hasConceptScore W4200605890C185592680 @default.
• W4200605890 hasConceptScore W4200605890C186460083 @default.
• W4200605890 hasConceptScore W4200605890C191897082 @default.
• W4200605890 hasConceptScore W4200605890C192562407 @default.

• next