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- W4205314949 abstract "Electrocatalytic reduction of N2 to ammonia (NH3) at ambient conditions has attracted widespread attention, and revealing the mechanism has been a remarkably challenging problem for decades. This work developed a low-cost and efficient multiple heteroatom codoped porous carbon catalyst from municipal sludge (MSB-P), which demonstrated excellent electrochemical stability and selectivity for the electrochemical N2 reduction reaction (N2RR). In 0.1 mol/L HCl solution, a high NH3 yield rate of 35.76 µg.h − 1.mg−1cat. and an excellent Faraday Efficiency (FE) of 7.79% at -0.7 V vs. RHE (reversible hydrogen electrode) were obtained under ambient conditions. Furthermore, the electrocatalytic mechanism of MSB-P for N2RR was also revealed by in situ Fourier transform infrared spectroscopy (FTIR) data, and an associative route was identified. These findings provide an exciting new method for fabricating inexpensive and efficient carbon-based catalysts for production of NH3 at ambient conditions." @default.
- W4205314949 created "2022-01-26" @default.
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- W4205314949 date "2022-03-01" @default.
- W4205314949 modified "2023-09-29" @default.
- W4205314949 title "Efficient electrocatalytic reduction of N2 to ammonia at ambient conditions with municipal sludge-derived porous carbon codoped with multiple heteroatoms" @default.
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- W4205314949 doi "https://doi.org/10.1016/j.electacta.2022.139934" @default.
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