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- W4205826763 abstract "Abstract We report herein an unprecedented gold and oxidative NHC relay catalysis that enables highly enantioselective cascade annulation between readily available α‐amino‐ynones with enals. This method utilizes the in situ ‐ generated pyrrolin‐4‐ones as a novel and versatile synthon, which engage with α,β‐unsaturated acylazolium intermediates generated from enals by oxidative NHC catalysis to produce pyrrole‐fused lactones in high yield and excellent enantioselectivity. Synthetic utility of the lactone products is also demonstrated by facile conversion to densely functionalized pyrroles and pyrrolin‐4‐ones in high yields with excellent stereopurity." @default.
- W4205826763 created "2022-01-26" @default.
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- W4205826763 date "2022-02-03" @default.
- W4205826763 modified "2023-09-27" @default.
- W4205826763 title "Enantioselective Cascade Annulation of α‐Amino‐ynones and Enals Enabled by Gold and Oxidative NHC Relay Catalysis" @default.
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- W4205826763 doi "https://doi.org/10.1002/ange.202115464" @default.
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