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• W4206151682 endingPage "2103622" @default.
• W4206151682 startingPage "2103622" @default.
• W4206151682 abstract "Rechargeable Zn–air batteries (ZABs) as high-energy density and cost-effective power sources for next generation energy storage have attracted considerable attention. However, the sluggish oxygen electrochemistry leads to high polarization of the air electrode during charge/discharge and consequently a low round-trip energy efficiency of the cell. Here it is shown that the two-electron oxygen redox chemistry enabled by a redox mediator, anthraquinone-2,7-disulfonic acid disodium salt (AQDS), can effectively boost the performance of ZABs. The kinetics and underlying mechanism of the AQDS-mediated oxygen reduction reaction at different pH are scrutinized both computationally and experimentally to delineate the reaction pathways and rate-limiting step. An ultrafast catalytic rate constant of 2.53 × 106 s–1 is achieved at a pH of 13.13 and based on a flow cell configuration, the AQDS-mediated Zn–air flow battery demonstrates considerably enhanced energy efficiency of 85% at 10 mA cm−2." @default.
• W4206151682 created "2022-01-26" @default.
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• W4206151682 date "2022-01-21" @default.
• W4206151682 modified "2023-09-29" @default.
• W4206151682 title "Redox‐Mediated Two‐Electron Oxygen Reduction Reaction with Ultrafast Kinetics for Zn–Air Flow Battery" @default.
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• W4206151682 doi "https://doi.org/10.1002/aenm.202103622" @default.
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