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• W4206210726 endingPage "134677" @default.
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• W4206210726 abstract "• CA-Cu nanozyme with both laccase- and catecholase-like activity is prepared. • A novel type of amorphous MOF (CA-Cu) is synthesized by the facile solvothermal reaction of cyanuric acid and Cu 2+ . • Compared with laccase, CA-Cu nanozyme has superior activity, stability and recyclability. • The higher degradation efficiency of CA-Cu nanozyme for environmental phenolic pollutants has been studied. • The enhancement of coordination between N and copper (N-Cu) for the laccase- and catecholase-like activity has been proved. In spite of the rapid development of nanozyme, it is still challenging to develop multifunctional nanozyme with high oxidase-like activity. In this work, a novel type of amorphous MOF based nanozyme (CA-Cu) with both laccase- and catecholase-like activity was prepared by the facile solvothermal reaction of cyanuric acid and Cu 2+ to mimick the N-Cu coordinated environment between the imidazole and Cu 2+ in their active site. Due to the excellent activity, substrate universality, recyclability and stability of CA-Cu nanozyme, it shows broad application prospects in degradation and detection of phenolic compounds. Besides, the structure–activity relationship between N-Cu coordinated environment and laccase/catecholase-like activity has been further proved." @default.
• W4206210726 created "2022-01-26" @default.
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• W4206210726 date "2022-04-01" @default.
• W4206210726 modified "2023-10-17" @default.
• W4206210726 title "Preparation of amorphous MOF based biomimetic nanozyme with high laccase- and catecholase-like activity for the degradation and detection of phenolic compounds" @default.
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• W4206210726 doi "https://doi.org/10.1016/j.cej.2022.134677" @default.
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