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- W4206326961 abstract "Solid-state sodium (Na) batteries (SSSBs) using sulfide-based solid electrolytes (SSEs) hold tremendous promise due to their high theoretical specific capacity, enhanced safety and abundant resources. However, detrimental interfacial issues between SSEs and Na metal present a major challenge to the advancement of sulfide-based SSSBs. To address interfacial issues, we demonstrate an efficient approach by incorporating an ionic liquid electrolyte ((PYR/Na)TFSI) as interlayer to stabilize the Na metal/SSE interface. The presence of the (PYR/Na)TFSI interlayer enables the formation of a stable solid electrolyte interphase (SEI) to prevent the harmful reactions and inhibit Na dendrites. Combination of ab initio molecular dynamics simulations and X-ray photoelectron spectroscopy reveale that this stable SEI is largely composed of reduced products of TFSI−, such as NaF and CF3. As a result, the symmetric cells exhibited stable Na plating/striping cycling for 300 h at 0.1 mA cm−2. In addition, FeS2||Na quasi-solid-state batteries delivered an impressive specific capacity of over 300 mAh g−1 under the current density of 20 mA g−1 at room temperature. Under a higher current density (100 mA g−1), such batteries performed with long-term cycling stability and maintained a specific capacity of around 103 mAh g−1 after 330 cycles. This work demonstrates the novel perspective of using an ionic liquid interlayer to address interfacial issues, contributing to the advancement of high-performance SSSBs for the next-generation energy storage systems." @default.
- W4206326961 created "2022-01-26" @default.
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- W4206326961 date "2022-04-01" @default.
- W4206326961 modified "2023-10-10" @default.
- W4206326961 title "Highly efficient interface stabilization for ambient-temperature quasi-solid-state sodium metal batteries" @default.
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- W4206326961 doi "https://doi.org/10.1016/j.cej.2022.134679" @default.
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