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- W4206446704 abstract "Conversion of CO2 into carbonaceous fuels with the aid of solar energy has been an important research subject for decades. Owing to their excellent electron-accepting capacities, fullerene derivatives have been extensively used as n-type semiconductors. This work reports that the fulleropyrrolidine functionalized with 4,7-di(thiophen-2-yl)benzo[c][1,2,5]thiadiazole, abbreviated as DTBT-C60 , could efficiently catalyze the photoreduction of CO2 to CO. The novel C60 -chromophore dyad structure facilitated better usage of solar light and effective dissociation of excitons. Consequently, the DTBT-C60 exhibited a promising CO yield of 144 μmol gcat-1 under AM1.5G solar illumination for 24 h. Moreover, the isotope experiments demonstrated that water molecules could function as an electron source to reactivate DTBT-C60 . Impressively, DTBT-C60 exhibited an extremely durable catalytic activity for more than one week, facilitating the practical application of photochemical CO2 reaction." @default.
- W4206446704 created "2022-01-25" @default.
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- W4206446704 date "2022-01-31" @default.
- W4206446704 modified "2023-09-25" @default.
- W4206446704 title "Chromatic Fulleropyrrolidine as Long‐Lived Metal‐Free Catalyst for CO<sub>2</sub> Photoreduction Reaction" @default.
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- W4206446704 doi "https://doi.org/10.1002/cssc.202102476" @default.
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