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- W4206667473 abstract "The transformations of monovalent thallium (Tl) in an aqueous environment may be affected significantly by Tl(I) partitioning at the solid-water interface during sorption. Models used to quantify the kinetics of Tl(I) adsorption on heterogeneous adsorbents and formation of multiple complexes under a wide range of water chemistry conditions can accurately predict the environmental fate of thallium. In this study, Tl(I) sorption on representative titanium dioxide at different solution pH values and loading concentrations was investigated with two unified adsorption models, diffuse layer modeling and kinetics modeling. Three Tl(I) surface complexes, TiOTl, TiOHTl+, and TiOTlOH-, were used in the diffuse layer model and successfully described batch adsorption and the results of spectroscopic analyses. The contribution of TiOHTl+ to the adsorption capacity was much higher than those of TiOTl and TiOTlOH- under neutral and weakly alkaline conditions, while the species TiOTlOH- predominated among Tl(I) complexes in strongly alkaline environments. The adsorption and desorption rate coefficients derived from thermodynamics and kinetics coupling modeling suggested the influence of different complex characteristics on adsorption and desorption of Tl(I). Our results provide a comprehensive model for predicting the dynamic binding behavior of Tl at heterogeneous solid-water interfaces." @default.
- W4206667473 created "2022-01-26" @default.
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- W4206667473 date "2022-04-01" @default.
- W4206667473 modified "2023-10-17" @default.
- W4206667473 title "Thermodynamic and kinetic coupling modeling for thallium(I) sorption at a heterogeneous titanium dioxide interface" @default.
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- W4206667473 doi "https://doi.org/10.1016/j.jhazmat.2022.128230" @default.
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