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• W4206678242 abstract "Due to the urgent need to reduce CO2 emission and the shortage of petroleum, using coals especially low-rank coals as raw materials for producing chemicals has attracted much attention. Thermal extraction and oxidation in aqueous solution are efficient approaches for obtaining oxygen-containing chemicals from low-rank coals. However, yield of chemicals is limited and/or large amount of CO2 is released solely using either of the two technologies for converting low-rank coals. In this paper, a low carbon footprint method combining thermal extraction (TE) and oxy-cracking in dilute alkali aqueous solution for efficiently depolymerizing three low-rank coals, i.e., Xiaolongtan lignite (XLT), Xilinguole lignite (XLGL), and Shenfu sub-bituminous coal (SF), was proposed. The results indicate that considerable oxygen-containing compounds such as phenols, esters, and humic acids along with little CO2 emission can be obtained via the two-step depolymerization process. TE temperature significantly effects the dissolution of small molecular compounds. Comparing with XLT and XLGL, SF has lower TE and oxy-cracking activity. A good correlation between the oxy-cracking conversion of TE residues and their DTG peak temperature for the low-rank coals can be found. Therefore, the aforementioned approach is promising for high-value and low-carbon utilization of low-rank coals." @default.
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• W4206678242 date "2022-05-01" @default.
• W4206678242 modified "2023-10-18" @default.
• W4206678242 title "A low carbon footprint method for converting low-rank coals to oxygen-containing chemicals" @default.
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• W4206678242 doi "https://doi.org/10.1016/j.fuel.2022.123277" @default.
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