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- W4206772783 abstract "Electrochemical hydrogenation (ECH) is a particularly important and environmentally friendly approach to obtain biomass-based fuels and high value-added fine chemicals without using external hydrogen. Herein, we reported a highly efficient and selective ECH of furfural (FF) into furfuryl alcohol (FA) with Cu-based electrocatalyst in aqueous alkaline media. Under the optimal conditions, FA selectivity close to 100% with 99% FF conversion and total Faradaic efficiency above 95% were obtained with the electrocatalyst. Mechanism investigation suggests an ECH mechanism for FA formation, which is highly potential-dependent to FA selectivity, requiring low and well-matched concentrations between active hydrogen (Hads) species and FA radical on the Cu surface. Moreover, the electrocatalyst shows an excellent stability and recyclability during the eight-time consecutive recycling experiments, yielding a total amount of 1011 mg FA. This work thus highlights an important guidance for electrocatalytic upgrading of biomass-based platform molecules in an environmentally friendly way." @default.
- W4206772783 created "2022-01-25" @default.
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- W4206772783 date "2022-05-01" @default.
- W4206772783 modified "2023-10-07" @default.
- W4206772783 title "Electrochemical hydrogenation of biomass-based furfural in aqueous media by Cu catalyst supported on N-doped hierarchically porous carbon" @default.
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- W4206772783 doi "https://doi.org/10.1016/j.apcatb.2022.121062" @default.
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