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- W4206809783 abstract "The p-type or n-type redox reactions of organics are being used as the reversible electrodes to build the next-generation rechargeable batteries with sustainable and tunable characteristics. However, the n-type organics that store cations generally exhibit low potential (<0.8 V vs. Zn/Zn2+), while the p-type organics that store anions suffer from limited capacity (<100 mAh g−1). Herein, we demonstrate that bis(phenylamino)phenothiazin-5-ium iodide (PTD-1) containing both n-type and p-type redox moieties exhibits a hybrid charge storage mechanism (n/p-type at low potential, p-type at high potential). Such a hybrid mechanism combines the advantages of n- and p-type reactions and compensates for the associated drawbacks of each. Accordingly, the aqueous Zn//PTD-1 full cell shows a high voltage (1.8 Vmaximum or 1.1 Vaverage), a high capacity 188.24 mAh gPTD-1−1 (achieved at 40 mA g−1), a long-life and a supercapacitor-like high power. These results shed new light on the design of advanced organic electrodes." @default.
- W4206809783 created "2022-01-25" @default.
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- W4206809783 date "2021-08-16" @default.
- W4206809783 modified "2023-10-17" @default.
- W4206809783 title "Molecular Tailoring of an n/p‐type Phenothiazine Organic Scaffold for Zinc Batteries" @default.
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- W4206809783 doi "https://doi.org/10.1002/ange.202106238" @default.
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