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- W4207020070 abstract "Flexible and rechargeable zinc–air batteries (ZABs) are promising energy sources for wearable electronic devices due to their high energy density and safe operation. However, the performance of quasi-solid-state electrolytes gradually degrades during the ion-exchange process, mainly because of water evaporation on the open cathode side, which reduces the lifespan of ZABs. Thus, a novel electrolyte needs to be designed that can retain water to increase the cycle lifespan of ZABs. Herein, we propose a near-neutral gel polymer electrolyte (GPE) composite comprising polyvinyl alcohol (PVA) and hydroxy-functionalized MXene. Benefiting from the three-dimensional porous network and numerous surface-functionalized hydroxy groups, the network of alkalized MXene inside the PVA matrix serves as a water reservoir, resulting in enhanced water retention, and therefore, a high ionic conductivity of 77.6 mS cm−1. The molecular dynamic simulations validate stronger hydrophilicity of alkalized MXene surface for water molecular than the pristine MXene. Resultantly, the assembled ZABs show a long cycle lifespan of 160 h at a current density of 2 mA cm−2 and a charging–discharging period of 15 min." @default.
- W4207020070 created "2022-01-26" @default.
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- W4207020070 date "2022-03-01" @default.
- W4207020070 modified "2023-10-16" @default.
- W4207020070 title "Gel polymer electrolyte with MXene to extend cycle lifespan of flexible and rechargeable Zinc–Air batteries" @default.
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- W4207020070 doi "https://doi.org/10.1016/j.jpowsour.2022.231020" @default.
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