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- W4207021225 abstract "Abstract The catalytic activity of a Ru complex 1 , bearing a fused π‐conjugated imidazo[1,2– a ][1,8]naphthyridine‐based mesoionic carbene (MIC) ligand, is examined for the oxidation of primary amines. Complex 1 affords nitrile or imine depending on the nature of the terminal oxidants and solvents used in the reactions. Primary amines are converted to nitriles using NaIO 4 in EtOAc/H 2 O mixture, whereas imines are obtained under O 2 balloon pressure in toluene. A variety of nitriles and imines are accessed with high yields and selectivity. A set of control experiments, reaction profiles, and kinetic studies are undertaken to disclose the mechanistic details for nitrile and imine formation. The catalytic reactions illustrate a subtle dependency on the choice of oxidants and solvents in the oxidation of primary amines." @default.
- W4207021225 created "2022-01-26" @default.
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- W4207021225 date "2022-01-23" @default.
- W4207021225 modified "2023-10-14" @default.
- W4207021225 title "Switchable activity of a Ru catalyst bearing an annulated mesoionic carbene ligand for oxidation of primary amines" @default.
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- W4207021225 doi "https://doi.org/10.1002/aoc.6594" @default.
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