FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4207029525> ?p ?o ?g. }

• W4207029525 endingPage "562" @default.
• W4207029525 startingPage "553" @default.
• W4207029525 abstract "Developing cost-effective and high-efficient bifunctional electrocatalyst for both oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) is essential for rechargeable Zn-air battery application. However, achieving high-active dual sites for bifunctional oxygen electrocatalysis in a single catalyst, as well as determining the decisive active sites for OER and ORR to explore the synergistically catalytic mechanism remain challenges. Herein, we propose a catalyst consisting of high-purity pyrrole nitrogen anchored cobalt single-atom (CoN4) and adjacent metallic cobalt sites (Cop@CoNC) for explicit research of dominated active sites. The obtained Cop@CoNC exhibits superior electrocatalytic activity with a small overpotential difference of 0.68 V between OER potential at 10 mA cm−2 and ORR half-wave potential, outperforming commercial noble-metal based catalysts. Electrochemical measurements and theoretical simulations verify the pyrrole-type CoN4 and adjacent metallic cobalt are separately decisive active sites for ORR and OER activities. Simultaneously, metallic cobalt regulates electron distribution of CoN4 moiety to improve ORR activity. Importantly, the rechargeable liquid and flexible solid-state Zn-air batteries using Cop@CoNC as air electrode catalysts possess high peak power densities of 188.8 and 121.8 mW cm−2, respectively. Our findings provide a feasible strategy to design high-performance multifunctional catalysts for rechargeable Zn-air batteries application." @default.
• W4207029525 created "2022-01-26" @default.
• W4207029525 creator A5031060635 @default.
• W4207029525 creator A5034670657 @default.
• W4207029525 creator A5082186187 @default.
• W4207029525 creator A5082360423 @default.
• W4207029525 date "2022-04-01" @default.
• W4207029525 modified "2023-09-30" @default.
• W4207029525 title "Designing superior bifunctional electrocatalyst with high-purity pyrrole-type CoN4 and adjacent metallic cobalt sites for rechargeable Zn-air batteries" @default.
• W4207029525 cites W1970127494 @default.
• W4207029525 cites W1979544533 @default.
• W4207029525 cites W2083222334 @default.
• W4207029525 cites W2092157292 @default.
• W4207029525 cites W2212773991 @default.
• W4207029525 cites W2511797146 @default.
• W4207029525 cites W2568897875 @default.
• W4207029525 cites W2611902734 @default.
• W4207029525 cites W2726465153 @default.
• W4207029525 cites W2735944262 @default.
• W4207029525 cites W2742325036 @default.
• W4207029525 cites W2759187213 @default.
• W4207029525 cites W2763659246 @default.
• W4207029525 cites W2784943348 @default.
• W4207029525 cites W2793756331 @default.
• W4207029525 cites W2806347718 @default.
• W4207029525 cites W2806882524 @default.
• W4207029525 cites W2808136178 @default.
• W4207029525 cites W2810922308 @default.
• W4207029525 cites W2884469847 @default.
• W4207029525 cites W2889270496 @default.
• W4207029525 cites W2902977219 @default.
• W4207029525 cites W2903795128 @default.
• W4207029525 cites W2933257288 @default.
• W4207029525 cites W2951311099 @default.
• W4207029525 cites W2961575260 @default.
• W4207029525 cites W2962552301 @default.
• W4207029525 cites W2985149168 @default.
• W4207029525 cites W2985474200 @default.
• W4207029525 cites W2990194258 @default.
• W4207029525 cites W2992071589 @default.
• W4207029525 cites W3000381939 @default.
• W4207029525 cites W3004138322 @default.
• W4207029525 cites W3006160935 @default.
• W4207029525 cites W3014910550 @default.
• W4207029525 cites W3023764478 @default.
• W4207029525 cites W3031569146 @default.
• W4207029525 cites W3039202373 @default.
• W4207029525 cites W3048454067 @default.
• W4207029525 cites W3049486162 @default.
• W4207029525 cites W3067283243 @default.
• W4207029525 cites W3091000417 @default.
• W4207029525 cites W3102940275 @default.
• W4207029525 cites W3105677887 @default.
• W4207029525 cites W3114432452 @default.
• W4207029525 cites W3122001600 @default.
• W4207029525 cites W3135856016 @default.
• W4207029525 cites W3136375870 @default.
• W4207029525 cites W3136741330 @default.
• W4207029525 cites W3160831603 @default.
• W4207029525 cites W3175299627 @default.
• W4207029525 cites W3184537369 @default.
• W4207029525 cites W3189177848 @default.
• W4207029525 cites W4236038718 @default.
• W4207029525 doi "https://doi.org/10.1016/j.ensm.2022.01.040" @default.
• W4207029525 hasPublicationYear "2022" @default.
• W4207029525 type Work @default.
• W4207029525 citedByCount "50" @default.
• W4207029525 countsByYear W42070295252022 @default.
• W4207029525 countsByYear W42070295252023 @default.
• W4207029525 crossrefType "journal-article" @default.
• W4207029525 hasAuthorship W4207029525A5031060635 @default.
• W4207029525 hasAuthorship W4207029525A5034670657 @default.
• W4207029525 hasAuthorship W4207029525A5082186187 @default.
• W4207029525 hasAuthorship W4207029525A5082360423 @default.
• W4207029525 hasConcept C127413603 @default.
• W4207029525 hasConcept C135473242 @default.
• W4207029525 hasConcept C147789679 @default.
• W4207029525 hasConcept C161790260 @default.
• W4207029525 hasConcept C17525397 @default.
• W4207029525 hasConcept C178790620 @default.
• W4207029525 hasConcept C179104552 @default.
• W4207029525 hasConcept C185592680 @default.
• W4207029525 hasConcept C186460083 @default.
• W4207029525 hasConcept C191897082 @default.
• W4207029525 hasConcept C192562407 @default.
• W4207029525 hasConcept C2780443040 @default.
• W4207029525 hasConcept C33989665 @default.
• W4207029525 hasConcept C42360764 @default.
• W4207029525 hasConcept C515602321 @default.
• W4207029525 hasConcept C52859227 @default.
• W4207029525 hasConceptScore W4207029525C127413603 @default.
• W4207029525 hasConceptScore W4207029525C135473242 @default.
• W4207029525 hasConceptScore W4207029525C147789679 @default.
• W4207029525 hasConceptScore W4207029525C161790260 @default.
• W4207029525 hasConceptScore W4207029525C17525397 @default.
• W4207029525 hasConceptScore W4207029525C178790620 @default.
• W4207029525 hasConceptScore W4207029525C179104552 @default.
• W4207029525 hasConceptScore W4207029525C185592680 @default.

• next