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• W4207029542 abstract "• Dual carriers based on metal–organic frameworks were first ever designed. • Excellent performance for CO/N 2 separation was obtained. • This study proposes a novel concept of “accelerated transport.” • The separation mechanism is delineated using molecular dynamic simulation. The significance of carbon monoxide (CO) as an invaluable starting material for chemical industries necessitates comprehensive analysis of membrane-based CO separation and recovery. In this regard, highly CO-selective mixed-matrix membranes (MMMs) based on dual carriers [Ag + ions and Ag nanoparticle (NP)-impregnated MIL-101 (Ag@MIL-101)] were fabricated herein for CO separation. A highly adhesive comb copolymer [poly(glycidyl methacrylate-co-poly(oxyethylene methacrylate); PGMA- co -POEM; PGO] plays a pivotal role as a di-functional matrix in anchoring Ag + ions and uniformly dispersing Ag@MIL-101 particles, resulting in excellent interfacial properties. An optimal CO-separation performance is achieved at an Ag@MIL-101 loading of 10 wt% (CO permeance of 30.7 GPU and CO/N 2 selectivity of 11.8), which is superior compared to that of membranes with single Ag + ions. This study elucidates the synergistic CO transport effect of the positively charged AgNP-impregnated MOFs and Ag + ions through the fabricated membranes, and proposes a novel concept of “accelerated transport.” The separation mechanism behind the high CO capture property is delineated using molecular dynamic simulation through morphology and energetic analyses." @default.
• W4207029542 created "2022-01-26" @default.
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• W4207029542 date "2022-05-01" @default.
• W4207029542 modified "2023-10-16" @default.
• W4207029542 title "Highly CO-Selective Mixed-Matrix membranes incorporated with Ag Nanoparticle-Impregnated MIL-101 Metal–Organic frameworks" @default.
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• W4207029542 doi "https://doi.org/10.1016/j.cej.2022.134803" @default.
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