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• W4207046277 abstract "Lithium (Li) has garnered considerable attention as an alternative anodes of next-generation high-performance batteries owing to its prominent theoretical specific capacity. However, the commercialization of Li metal anodes (LMAs) is significantly compromised by non-uniform Li deposition and inferior electrolyte-anode interfaces, particularly at high currents and capacities. Herein, a hierarchical three-dimentional structure with CoSe2 -nanoparticle-anchored nitrogen-doped carbon nanoflake arrays is developed on a carbon fiber cloth (CoSe2 -NC@CFC) to regulate the Li nucleation/plating process and stabilize the electrolyte-anode interface. Owing to the enhanced lithiophilicity endowed by CoSe2 -NC, in situ-formed Li2 Se and Co nanoparticles during initial Li nucleation, and large void space, CoSe2 -NC@CFC can induce homogeneous Li nucleation/plating, optimize the solid electrolyte interface, and mitigate volume change. Consequently, the CoSe2 -NC@CFC can accommodate Li with a high areal capacity of up to 40 mAh cm-2 . Moreover, the Li/CoSe2 -NC@CFC anodes possess outstanding cycling stability and lifespan in symmetric cells, particularly under ultrahigh currents and capacities (1600 h at 10 mA cm-2 /10 mAh cm-2 and 5 mA cm-2 /20 mAh cm-2 ). The Li/CoSe2 -NC@CFC//LiFePO4 full cell delivers impressive long-term performance and favorable flexibility. The developed CoSe2 -NC@CFC provides insights into the development of advanced Li hosts for flexible and stable LMAs." @default.
• W4207046277 created "2022-01-26" @default.
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• W4207046277 date "2022-01-24" @default.
• W4207046277 modified "2023-10-01" @default.
• W4207046277 title "Achieving Uniform Li Plating/Stripping at Ultrahigh Currents and Capacities by Optimizing 3D Nucleation Sites and Li ₂ Se‐Enriched SEI" @default.
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• W4207046277 doi "https://doi.org/10.1002/advs.202104689" @default.
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