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• W4207047478 endingPage "1263" @default.
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• W4207047478 abstract "In this chapter, we will outline the development of using CO 2 as –CH– and –CH 2 – sources through two-electron or four-electron reductive functionalization of CO 2 , respectively. The main routes of these transformations consist of two/four electrons that reduce CO 2 to C (+2) or C (0) active intermediates and sequent bonding reactions with nucleophiles or transition-metal catalytic process. We focus on the homogeneous reductive transformation of CO 2 with extra coupling partners. The self-reduction of CO 2 to give reductive C1 compounds (CO, HCHO, HCOOH, C, CH 4 , etc.) or construct higher alcohols, aromatics, and the six-electron reduction of CO 2 as methylation reagents will not be discussed here. After a brief introduction of the importance and challenges in using CO 2 as –CH– and –CH 2 – sources by controllable CO 2 reduction, the development of reductive transformations of CO 2 by versatile catalytic systems with different bonding types will be discussed in detail both in reaction scopes and mechanisms. Finally, a summary and outlook of this area will be presented." @default.
• W4207047478 created "2022-01-26" @default.
• W4207047478 creator A5005864134 @default.
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• W4207047478 date "2022-01-21" @default.
• W4207047478 modified "2023-10-12" @default.
• W4207047478 title "Using <scp>CO</scp> ₂ as – <scp>CH</scp> – and – <scp>CH</scp> ₂ – Sources" @default.
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