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• W4207048323 abstract "In this work, a cylindrical flow-through electro-Fenton reactor containing graphite felt electrodes and an Fe(II) loaded resin was evaluated for the production of the Fenton reaction mixture and for the degradation of amoxicillin (AMX) and fecal coliforms containing aqueous solutions. First, the influence of several factors such as treatment time, current intensity, flow rate, and electrode position was investigated for the electrogeneration of H2O2 and the energetic consumption by means of a factorial design methodology using a 24 factorial matrix. Electric current and treatment time were found to be the pivotal parameters influencing the H2O2 production with contributions of 40.2 and 26.9%, respectively. The flow rate had low influence on the responses; however, 500 mL min-1 (with an average residence time of 1.09 min obtained in the residence time distribution analysis) allowed to obtain a better performance due to the high mass transport to and from the electrodes. As expected, polarization was also found to play an important role, since for the cathode-to-anode flow direction, lower H2O2 concentrations were observed when compared with the anode-to-cathode flow arrangement, indicating that part of the H2O2 produced in the cathode was destroyed at the anode. A fluorescence study of hydroxyl radical production, on the other hand, showed that higher yields were obtained using an anode-to-cathode flow direction (up to 3.88 µM), when compared with experiments carried out using a cathode-to-anode flow path (3.11 µM). The removal of a commercial formulation of the antibiotic AMX was evaluated in terms of total organic carbon, achieving up to 57.9% and 38.63% of pollutant mineralization using synthetic and real sanitary wastewater spiked, respectively. Finally, the efficiency of the process on the inactivation of fecal coliforms in sanitary wastewater samples was assessed, reducing 90% of the bacteria after 5 min of electrolysis." @default.
• W4207048323 created "2022-01-26" @default.
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• W4207048323 date "2022-01-25" @default.
• W4207048323 modified "2023-10-18" @default.
• W4207048323 title "Study of the performance of a cylindrical flow-through electro-Fenton reactor using different arrangements of carbon felt electrodes: effect of key operating parameters" @default.
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• W4207048323 doi "https://doi.org/10.1007/s11356-021-18118-6" @default.
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