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- W4207050359 abstract "Abstract Access to block copolymers from monomers that do not polymerize via a common mechanism requires initiation from a multifunctional species that allows orthogonal polymerization chemistries. We disclose a strategy to provide well‐defined polyacrylamido‐ b ‐polyether block copolymers by a one‐pot combination of photoiniferter polymerization and organocatalytic ring‐opening polymerization (ROP) using a hydroxy‐functionalized trithiocarbonate photoiniferter as the dual initiator at ambient temperature. Our results reveal good compatibility between the two polymerization systems and highlight that they can be performed in arbitrary order or simultaneously with good retention of the thiocarbonylthio functionality. We also demonstrate selective temporal control over the photoiniferter polymerization during concurrent ROP. We harnessed the efficiency of combining these polymerization systems to provide tailor‐made block copolymers from chemically distinct monomers." @default.
- W4207050359 created "2022-01-26" @default.
- W4207050359 creator A5019879013 @default.
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- W4207050359 date "2021-07-14" @default.
- W4207050359 modified "2023-10-18" @default.
- W4207050359 title "Hybrid Block Copolymer Synthesis by Merging Photoiniferter and Organocatalytic Ring‐Opening Polymerizations" @default.
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- W4207050359 doi "https://doi.org/10.1002/ange.202106418" @default.
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