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- W4207059410 abstract "Abstract 2D metal–organic‐framework (MOF) based composites have emerged as promising candidates for electrocatalysis due to their high structural flexibility and fully exposed active sites. Herein, a freestanding metal–organic layer (MOL) with a 2D kgd (kagome dual) lattice was constructed with abundant surface oxygenate groups serving as anchoring sites to immobilize diverse guests. Taking Bi as an example, tetragonal Bi 2 O 3 nanowires can be uniformly grown on MOLs after solvothermal treatment, the structural evolution of which was followed by ex situ electron microscopy. The as‐prepared Bi 2 O 3 /MOL exhibits excellent CO 2 electroreduction activity towards formate reaching a specific current of 2.3 A mg Bi −1 and Faradaic efficiencies of over 85 % with a wide potential range from −0.87 to −1.17 V, far surpassing Bi 2 O 3 /UiO (a 3D Zr 6 ‐oxo based MOF) and Bi 2 O 3 /AB (Acetylene Black). Such a post‐synthetic modification strategy can be flexibly extended to develop versatile MOL composites, highlighting the superiority of optimizing MOL‐based composites for electrocatalysis." @default.
- W4207059410 created "2022-01-26" @default.
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- W4207059410 date "2022-01-18" @default.
- W4207059410 modified "2023-10-16" @default.
- W4207059410 title "Assembling Metal Organic Layer Composites for High‐Performance Electrocatalytic CO 2 Reduction to Formate" @default.
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- W4207059410 doi "https://doi.org/10.1002/ange.202117058" @default.
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