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- W4207063870 abstract "Elaborate molecular design on cathodes is of great importance for rechargeable aqueous zinc-organic batteries' performance elevation. Herein, we design a novel orthoquinone-based covalent organic framework with an ordered channel structures (BT-PTO COF) cathode for an ultrahigh performance aqueous zinc-organic battery. The ordered channel structure facilitates ions transfer and makes the COF follow a redox pseudocapacitance mechanism. Thus, it delivers a high reversible capacity of 225 mAh g-1 at 0.1 A g-1 and an exceptional long-term cyclability (retention rate 98.0 % at 5 A g-1 (≈18 C) after 10 000 cycles). Moreover, a co-insertion mechanism with Zn2+ first followed by two H+ is uncovered for the first time. Significantly, this co-insertion behaviour evolves to more H+ insertion routes at high current density and gives the COF ultra-fast kinetics thus it achieves unprecedented specific power of 184 kW kg-1(COF) and a high energy density of 92.4 Wh kg-1(COF) . Our work reports a superior organic material for zinc batteries and provides a design idea for future high-performance organic cathodes." @default.
- W4207063870 created "2022-01-26" @default.
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- W4207063870 date "2022-02-03" @default.
- W4207063870 modified "2023-10-16" @default.
- W4207063870 title "Orthoquinone–Based Covalent Organic Frameworks with Ordered Channel Structures for Ultrahigh Performance Aqueous Zinc–Organic Batteries" @default.
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- W4207063870 doi "https://doi.org/10.1002/anie.202117511" @default.
- W4207063870 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35064728" @default.
- W4207063870 hasPublicationYear "2022" @default.