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- W4207066208 abstract "Herein, we attempt to regulate the growth of the primary grains and internal structure of the secondary particles of Li[Ni0.88Co0.09Al0.03]O2 through synthesis calcination temperature. It is revealed that the interval space generated by the packing of the primary grains in the secondary particles is strongly dependent on the calcination temperature in a relative narrow temperature region (700–800 °C) and plays a key role in maintaining the integrity of the secondary particles during electrochemical cycling. Rich interval space in the samples obtained at low calcination temperature (700 °C) endows the materials with superior cycling stability and rate capability, due to the improvement of the ability to buffer the stress induced by repeated volume change of the crystal lattice and the accessibility of the electrolyte of the material during cycling. In particular, this might efficiently avoid the fracture of the secondary particles as that occurs for the samples with densely packed primary grains obtained at high calcination temperature (800 °C). Based on the findings, a facile approach by simple adjustment of the calcination temperature is developed to optimize the microstructure of the material to provide reasonable cycling and rate performance." @default.
- W4207066208 created "2022-01-26" @default.
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- W4207066208 date "2022-03-01" @default.
- W4207066208 modified "2023-09-27" @default.
- W4207066208 title "Improvement of electrochemical performance of nickel-rich LiNi0.88Co0.09Al0.03O2 through calcination regulation of primary grains" @default.
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- W4207066208 doi "https://doi.org/10.1016/j.jpowsour.2022.231044" @default.
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