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- W4207076274 abstract "We report high-pressure (up to 50 MPa) ESR-spectroscopic investigations on the rotational correlation times of the nitroxide radicals 2,2,6,6-tetramethylpiperidine 1-oxyl (TEMPO), 4-hydroxy-2,2,6,6-tetramethylpiperidine 1-oxyl (TEMPOL), and 4-amino-2,2,6,6-tetramethylpiperidine 1-oxyl (ATEMPO) in the ionic liquids 1-ethyl-3-methylimidazolium tetrafluoroborate (emimBF4), 1-butyl-3-methylimidazolium hexafluorophosphate (bmimPF6), 1-butyl-3-methylimidazolium tetrafluoroborate (bmimBF4), 1-methyl-3-octylimidazolium tetrafluoroborate (omimBF4), and 1-methyl-3-octylimidazolium hexafluorophosphate (omimPF6). The activation volumes (38.5-56.6 Å3) determined from pressure dependent rotational diffusion coefficients agree well with the pressure dependent viscosities of the ionic liquids. Experimentally, the fractional exponent of the generalized Stokes-Einstein-Debye relation is found to be close to one." @default.
- W4207076274 created "2022-01-26" @default.
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- W4207076274 date "2022-01-24" @default.
- W4207076274 modified "2023-09-29" @default.
- W4207076274 title "High-Pressure ESR Spectroscopy: On the Rotational Motion of Spin Probes in Pressurized Ionic Liquids" @default.
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- W4207076274 doi "https://doi.org/10.1021/acs.jpcb.1c09243" @default.
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