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• W4210273959 endingPage "134927" @default.
• W4210273959 startingPage "134927" @default.
• W4210273959 abstract "• Thermal decomposition of NCM families is followed by Avrami-Erofeev mechanism. • Phase transition contributes to determinative exothermic reaction for instability. • Single-crystalline NCM shows less thermal stability than poly-crystalline one. Insufficient thermal stabilities of LiNi x Co y Mn 1-x-y O 2 (NCM) families have aroused wide concerns and safety threats against large-scale application due to oxygen releasing and exothermic side reactions. Towards energy-dense batteries, single-crystalline NCM has been recently highlighted as a promising substitution in providing improved capacity retention beyond polycrystalline counterparts. However, their thermal-driven degradation mechanism remains under investigation and yet critically essential. In this contribution, we have rationally explored the thermal-driven fading behavior of delithiated single-crystalline and polycrystalline LiNi 0.88 Co 0.07 Mn 0.05 O 2 . Followed by the Avrami-Erofeev mechanism, a three-step decomposition procedure has been deconvoluted from time-resolved X-ray diffraction and physicochemical analysis, in terms of solid electrolyte interface (SEI) decomposition, layered-to-spinel transition and spinel-to-rock-salt transition. According to thermal kinetic analysis, polycrystalline LiNi 0.88 Co 0.07 Mn 0.05 O 2 exhibits higher decomposition temperature and lower decomposition rate than that in single-crystalline counterparts, contributing to better thermal stability. This study has provided a fundamental understanding of the thermal decomposition of Ni-rich LiNi 0.88 Co 0.07 Mn 0.05 O 2 cathodes and insights of NCM families protection." @default.
• W4210273959 created "2022-02-08" @default.
• W4210273959 creator A5071082922 @default.
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• W4210273959 date "2022-05-01" @default.
• W4210273959 modified "2023-10-18" @default.
• W4210273959 title "Unveiling thermal decomposition kinetics of Single-Crystalline Ni-Rich LiNi0.88Co0.07Mn0.05O2 cathode for safe Lithium-Ion batteries" @default.
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• W4210273959 doi "https://doi.org/10.1016/j.cej.2022.134927" @default.
• W4210273959 hasPublicationYear "2022" @default.
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