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- W4210274633 abstract "Synthetic systems of nonequilibrium self-assembly have made considerable progress; however, the achievement of innovative materials with self-regulated functions analogous to living systems remains a grand challenge. Herein, a versatile nonequilibrium system of polymer brushes with spatiotemporally programmable properties and functions driven by chemical fuels is reported. By combining a responsive polymer with an autonomous pH regulator, the polymer brushes self-regulate their swelling and deswelling process with tunable lifetimes. By using patterned copolymer brushes with pH-responsive fluorescence moiety, an autonomous fluorescence modulator is created that self-regulates its fluorescence in spatiotemporally programmable fashion driven by a chemical or an enzymatic reaction. Furthermore, a self-regulated wettability switcher of polymer brushes both in air and in an aqueous solution is implemented. The methodology and results in the work provide a useful avenue into the exploration of nonequilibrium synthetic materials with programmable functions and would accelerate the transformative developments of nonequilibrium materials and systems in practical applications." @default.
- W4210274633 created "2022-02-08" @default.
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- W4210274633 date "2022-02-04" @default.
- W4210274633 modified "2023-09-28" @default.
- W4210274633 title "Chemical Fuel Mediated Self‐Regulatory Polymer Brushes for Autonomous Fluorescence Modulator and Wettability Switcher" @default.
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- W4210274633 doi "https://doi.org/10.1002/marc.202100878" @default.
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