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• W4210291220 endingPage "5095" @default.
• W4210291220 startingPage "5079" @default.
• W4210291220 abstract "Photocatalytic degradation is a sustainable technique for reducing the environmental hazards created by the overuse of antibiotics in the food and pharmaceutical industries. Herein, a layer of MoS2/g-C3N4 nanocomposite is introduced to zirconium oxide (ZrO2) nanoparticles to form a particle-embedded-layered structure. Thus, a narrow band gap (2.8 eV) starts developing, deliberated as a core photodegradation component. Under optimization, a high photocatalytic activity of 20 mg/L TC at pH 3 with ZrO2@MoS2/g-C3N4 nanocomposite was achieved with 94.8% photocatalytic degradation in 90 min. A photocatalytic degradation rate constant of 0.0230 min-1 is determined, which is 2.3 times greater than the rate constant for bare ZrO2 NPs. The superior photocatalytic activity of ZrO2@MoS2/g-C3N4 is due to the dual charge-transfer channel between the MoS2/g-C3N4 and ZrO2 nanoparticles, which promotes the formation of photogenerated e-/h+ pairs. Charge recombination produces many free electron-hole pairs, which aid photocatalyst reactions by producing superoxide and hydroxyl radicals via electron-hole pair generation. The possible mechanistic routes for TC were investigated in-depth, as pointed out by the liquid chromatography-mass spectrometry (LC-MS) investigation. Overall, this work shows that photocatalysis is a feasible sorbent approach for environmental antibiotic wastewater treatment." @default.
• W4210291220 created "2022-02-08" @default.
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• W4210291220 date "2022-02-02" @default.
• W4210291220 modified "2023-09-26" @default.
• W4210291220 title "Promoting Spatial Charge Transfer of ZrO₂ Nanoparticles: Embedded on Layered MoS₂/g-C₃N₄ Nanocomposites for Visible-Light-Induced Photocatalytic Removal of Tetracycline" @default.
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• W4210291220 doi "https://doi.org/10.1021/acsomega.1c06089" @default.
• W4210291220 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35187324" @default.
• W4210291220 hasPublicationYear "2022" @default.
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