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- W4210296357 abstract "In this study, we reported a hydrogen-bond-donor-directed enantiodivergent vinylogous aldol-cyclization cascade reaction of 3-alkylidene oxindoles with isatins and o-quinones. Both enantiomers can be prepared by thiourea or squaramide cinchona alkaloid bifunctional organocatalysts with the same quinine scaffold. Kinetic study data provided the possible reaction mechanism for the vinylogous aldol-cyclization cascade reaction. The DFT calculation data showed the geometry of the generated dienolates from pronucleophiles dominated the observed switch of enantioselectivity." @default.
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- W4210296357 date "2022-01-27" @default.
- W4210296357 modified "2023-10-14" @default.
- W4210296357 title "Hydrogen-Bond-Donor-Directed Switching of Enantioselectivity in the Vinylogous Aldol–Cyclization Cascade Reaction of Prostereogenic 3-Alkylidene Oxindoles with Isatins and <i>o</i>-Quinones" @default.
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- W4210296357 doi "https://doi.org/10.1021/acs.joc.1c02421" @default.
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