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• W4210488943 abstract "The development of high-performance solid polymer electrolytes is crucial for producing all-solid-state lithium metal batteries with high safety and high energy density. However, the low ionic conductivity of solid polymer electrolytes and their unstable electrolyte/electrode interfaces have hindered their widespread utilization. To address these critical challenges, a strong Lewis acid (aluminum fluoride (AlF3)) with dual functionality is introduced into polyethylene oxide) (PEO)-based polymer electrolyte. The AlF3 facilitates the dissociation of lithium salt, increasing the iontransfer efficiency due to the Lewis acid-base interaction; further the in-situ formation of lithium fluoride-rich interfacial layer is promoted, which suppresses the uneven lithium deposition and continuous undesired reactions between the Li metal and PEO matrix. Benefiting from our rational design, the symmetric Li/Li battery with the modified electrolyte exhibits much longer cycling stability (over 3600 h) than that of the pure PEO/lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) electrolyte (550 h). Furthermore, the all-solid-state LiFePO4 full cell with the composite electrolyte displays a much higher Coulombic efficiency (98.4% after 150 cycles) than that of the electrolyte without the AlF3 additive (63.3% after 150 cycles) at a large voltage window of 2.4–4.2 V, demonstrating the improved interface and cycling stability of solid polymer lithium metal batteries." @default.
• W4210488943 created "2022-02-08" @default.
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• W4210488943 date "2022-01-10" @default.
• W4210488943 modified "2023-10-01" @default.
• W4210488943 title "A strong Lewis acid imparts high ionic conductivity and interfacial stability to polymer composite electrolytes towards all-solid-state Li-metal batteries" @default.
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• W4210488943 doi "https://doi.org/10.1007/s40843-021-1908-x" @default.
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