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• W4210508712 abstract "Abstract Herein, a general approach to intermolecular benzylic C(sp 3 )−H alkylation of methyl‐substituted arenes is reported using metal carbenes derived from N ‐aryl‐α‐diazo‐β‐amidoesters and dirhodium catalysts. Alkylated products were formed in up to 81 % yield with demonstrated functional group tolerance, outpacing previous literature. The unique amide‐ester scaffolding can be exploited through various derivatizations for broad synthetic utility and provides a starting point for the development of selectivity rules and reactivity profiles for these intermolecular C(sp 3 )−H functionalizations." @default.
• W4210508712 created "2022-02-08" @default.
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• W4210508712 date "2022-03-14" @default.
• W4210508712 modified "2023-09-26" @default.
• W4210508712 title "Rh(II)‐catalyzed Intermolecular Benzylic C(sp³)−H Alkylation of Methyl‐substituted Arenes by <i>N</i>‐Aryl‐α‐diazo‐β‐amidoesters" @default.
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• W4210508712 doi "https://doi.org/10.1002/cctc.202101977" @default.
• W4210508712 hasPublicationYear "2022" @default.
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