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- W4210524325 abstract "Self-assembly of two-dimensional (2D) nanosheets into three-dimensional (3D) aerogels, can solve the problems of recovery and re-stacking, and fully utilize the potential of high specific surface areas and easily accessible surface sites. However, organic binders have to be added to fabricate aerogels using 2D nanosheets as building blocks, which inevitably limit the performance of 2D nanosheets due to covered surfaces. Herein, we proposed a new strategy to fabricate vermiculite aerogels (VAs) assembled from delaminated vermiculite nanosheets (VNSs) via metal ion induced fast gelation. The cheap and earth-abundant vermiculite was used as the raw materials to produce high-quality nanosheets by high speed shear-mixing. VNSs with a concentration as high as 15 mg/mL were produced. The concentration-dependent gelation performance was studied and showed a critical concentration of 6 mg/mL for gelation and fabricating monolithic aerogels without cracks. It is also found metal ions played critical roles in formation mechanically stable and robust aerogels with trivalent cations, particularly Al3+ being most effective. The edge-surface intertwining VNSs induced by the Al3+ cross-linking endow the VAs good mechanical strength and excellent environmental stability. As fixed adsorbent beds, the VAs show promising performance in fast removing organic dyes from water due to the developed pore structures, large specific surface area, and exposed surface sites." @default.
- W4210524325 created "2022-02-08" @default.
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- W4210524325 date "2022-03-01" @default.
- W4210524325 modified "2023-10-13" @default.
- W4210524325 title "Vermiculite aerogels assembled from nanosheets via metal ion induced fast gelation" @default.
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- W4210524325 doi "https://doi.org/10.1016/j.clay.2022.106431" @default.
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