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• W4210556022 abstract "Ruddlesden-popper (La, Sr)FeO4+δ perovskite oxide with excellent redox stability shows insufficient electrochemical catalytic activity for CO2 reduction because of low conductivity and oxygen vacancy concentration. In this work, Ni modified (La, Sr)Fe1-xNixO4+δ cathode was developed to improve the conductivity and catalytic activity for CO2 electrolysis. The introduction of the Ni element significantly increases the conductivity of (La, Sr)FeO4+δ perovskite oxide in both air and 50%CO2/CO due to the increasing charge carrier's concentration. Furthermore, the symmetric cell with (La, Sr)Fe0·9Ni0·1O4+δ (RPLSFNi0.1) electrode exhibits the lowest polarization resistance in 50%CO2/CO, suggesting that the RPLSFNi0.1 electrode has the best catalytic activity for CO2 electrolysis. Moreover, the addition of Sm0.2Ce0·8O2-δ (SDC) in RPLSFNi0.1 electrode further enhances the electrochemical performance, and the current density of −1170 mA cm−2 is obtained at 850 °C and 1.5 V. In addition, the electrolysis cell exhibits excellent reversible cycling operating stability between 0.6 V at fuel cell mode and 1.2 V at electrolysis mode, indicating that RPLSFNi0.1 is a robust cathode material for solid oxide cells (SOCs) fuel electrode." @default.
• W4210556022 created "2022-02-08" @default.
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• W4210556022 date "2022-02-01" @default.
• W4210556022 modified "2023-10-14" @default.
• W4210556022 title "Robust Ni-doped Ruddlesden-popper (La,Sr)Fe1-xNixO4+δ oxide as solid oxide cells fuel electrode for CO2 electrolysis" @default.
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• W4210556022 doi "https://doi.org/10.1016/j.ijhydene.2022.01.054" @default.
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